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个人简介
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教育经历
2013/09―2019/06 厦门大学，物理化学，理学博士
指导教师：孙世刚 教授，王朝晖 教授
2009/09―2013/07 厦门大学，化学，理学学士
工作经历
2025/03―至今 东南大学，化学化工学院，副研究员
2021/09―2025/02 犹他州立大学，化学与化学生物学系，博士后研究员
博士后合作导师：Yi Rao, Associate Professor
2019/07―2021/06 厦门大学，化学系，科研助理
皇甫至超，男，1992年4月生。聚焦复杂界面体系的结构与动力学的研究，发展了新的非线性光谱技术：1）搭建了原位和频光谱系统，研究了关键电化学界面过程，准确提取了电化学界面吸附物种分子水平的信息；2）发展了针对光电极等高性能二维材料电子表面态的研究方法，成功用于探测电子表面态的能量、谱学相位、动力学等信息，有助于全面理解其性质和在光催化反应中的作用；3）发展了基于飞秒脉冲整形器的界面特异性二维光谱方法，实现了复杂界面体系激发态动力学、能量耦合机制的直接探测，加深了对高性能材料界面过程的理解。已发表SCI期刊论文34篇，包含J. Am. Chem. Soc.，Angew. Chem. Int. Ed.，Laser Photonics Rev.，JACS Au，J. Phys. Chem. Lett.，J.Chem. Phys.等15篇第一或共一或通讯作者身份文章。
2025年3月加入东南大学化学化工学院游雨蒙教授团队，主要研究方向是非线性光谱方法用于极性材料性质和表界面过程的表征。
谷歌学术：https://scholar.google.com/citations?user=OOOt6zsAAAAJ
代表性文章
# denotes equally-contributed author, * denotes corresponding author1. Fan, C.-C.;* Jiao, S.-L.; Bi, Q.-Q.; Wu, J.-H.; Fu, H.-L.; Liu, C.-D.; Du, G.-W.; Huang-Fu,Z.-C.;* Wang, W.*, Chiral Nonlinear Optical Response in AchiralQuasi-2D Perovskite Ferroelectric Featuring Unusually Large A-Site Cation. Angew.Chem. Int. Ed. 2026, e3136861.
2. Cao,X.-X.; Du, G.-W.; Zhang, X.-Z.; Zhou, R.-J.; Sha, T.-T.; Pan, Q.; Huang-Fu,Z.-C.;* You, Y.-M.*, Multiple Ferroelectric-Polarization-DependentCouplings and Stable Modulation of Nonlinear Light in 2D Material/FerroelectricVan Der Waals Heterostructures. LaserPhotonics Rev. 2026, e02682.
3. Huang-Fu, Z.-C.;# Qian, Y.;# Brown, J. B.; Rao, Y.*, Orientational and Solvent Couplings of Molecules at Interfaces by Interface-Specific Two-Dimensional Vibrational-Electronic(i2D-VE) Spectroscopy. J. Phys. Chem.Lett. 2025, 16 (29), 7451-7461.
4. Wang, H.; Fisher, H.; Huang-Fu, Z.-C.;* Brown,J. B.; Zhang, T.; Song, F.; Qian, Y.; Rao, Y.*, Orientational Geometry, Surface Density, and Binding Free Energy of Intermediates as Full Descriptors for Electrochemical CO2 Reduction at Metal Surfaces. J. Am. Chem. Soc. 2025, 147 (22), 19101-19112.
5. Huang-Fu, Z.-C.;# Zhang, T.;# Brown, J. B.; Qian, Y.; Fisher, H.; Rao, Y.*, In-plane Orientational Motions of the Functional Groups of Molecules at the Air/Water Interface by Time-Resolved Vibrational Sum Frequency Generation. J. Chem. Phys. 2024, 161 (16), 164711.
6. Qian, Y.;# Huang-Fu, Z.-C.;# Li H.;# Zhang, T.;# Li, X.; Schmidt, S.; Fisher, H.; Brown,J. B.; Harutyunyan, A. R.; Chen, H.;* Chen, G.;* Rao, Y.*, Room-Temperature Halide Perovskites-Based Short-Wave IR Detectors with High Responsivity and Ultrabroad Bandwidth. JACS Au 2024, 4 (10),3921–3930.
7. Huang-Fu, Z.-C.; Qian, Y.; Zhang, T.;Brown, J. B.; Rao, Y.*, Development of Phase-Cycling Interface-Specific Two-Dimensional Electronic Sum Frequency Generation (2D-ESFG) Spectroscopy. J.Chem. Phys. 2024, 161 (11), 114201.
8. Huang-Fu, Z.-C.;# Tkachenko N.V.;# Qian, Y.;# Zhang, T.; Brown, J. B.; Harutyunyan, A.R.; Chen, G.; Rao, Y.*, Conical Intersections at Interfaces Revealed by Phase-Cycling Interface-Specific Two-Dimensional Electronic Spectroscopy(i2D-ES). J. Am. Chem. Soc. 2024, 146 (30), 20996-21007.
9. Zhang, T.; Brown, J. B.; Fisher, H.; Liebes, M.; Huang-Fu,Z.-C.;* Qian, Y.; Rao, Y.*, Surface states of photoelectrodes by surface-specific steady-state and time-resolved sum frequency spectroscopies. Chin. J. Chem. Phys. 2024, 37 (3), 376-397.
10. Huang-Fu, Z.-C.;# Qian, Y.;# Zhang, T.; Deng, G. H.; Brown, J. B.; Fisher, H.; Schmidt, S.; Chen, H.; Rao,Y.*, Orientational Coupling of Molecules at Interfaces Revealed by Two-Dimensional Electronic-Vibrational Sum Frequency Generation (2D-EVSFG). JACS Au 2023, 3 (5), 1413-1423.
11. Huang-Fu, Z.-C.; Qian, Y.; Deng, G. H.;Zhang, T.; Schmidt, S.; Brown, J.; Rao, Y.*, Development of Two-Dimensional Electronic-Vibrational Sum Frequency Generation (2D-EVSFG) for Vibronic and Solvent Couplings of Molecules at Interfaces and Surfaces. ACS Phys. Chem. Au 2023,3 (4), 374-385.
12. Zhang, T.;# Huang-Fu, Z.-C.;# Qian, Y.; Gao, H.;* Brown, J. B.; Rao, Y.*, Photoinduced Surface Electric Fields and Surface Population Dynamics of GaP(100) Photoelectrodes. J. Phys. Chem.C 2022, 126 (14), 6531-6541.
13. Qian, Y.;# Huang-Fu, Z.-C.;# Zhang, T.; Li, X.; Harutyunyan, A. R.;Chen, G.; Chen, H.;* Rao, Y.*, Temperature-Dependent Recombination of Triplet Biexcitons in Singlet Fission of Hexacene. J.Phys. Chem. C 2022, 126 (19), 8377-8383.
14. Huang-Fu, Z.-C.; Song, Q.-T.;He, Y.-H.; Liu, X.-L.; Wang, J.-J.; Sun, S.-G.;* Wang, Z.-H.*, Surface configuration of CO adsorbed on nanostructured Pt electrodes probed using broadband sum frequency generation spectroscopy. Chem. Commun. 2020, 56 (67), 9723-9726.
15. Huang-Fu, Z.-C.; Song, Q.-T.;He, Y.-H.; Wang, J.-J.; Ye, J.-Y.; Zhou, Z.-Y.; Sun, S.-G.;* Wang, Z.-H.*, Electrochemical CO2 reduction on Cu and Au electrodes studied using in situ sum frequency generation spectroscopy. Phys.Chem. Chem. Phys. 2019, 21 (45), 25047-25053.
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